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High-pressure scanning tunnelling microscopy (HP-STM) was used to study the room temperature adsorption of CO on a Pt(111) single crystal surface in equilibrium with the gas phase. The coverage was found to vary continu- ously, and over the entire range from 10 ¡6 {760 Torr pressure-dependent moire patterns were observed, characteristic of a hexagonal or nearly hexagonal CO overlayer. Two difierent pressure ranges can be distinguished: below 10 ¡2 Torr

High-Coverage Structures of Carbon Monoxide Adsorbed on Pt(111) Studied by High-Pressure Scanning Tunneling Microscopy