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The permeation, rejection, and transport of electrolytes in water-fillednanopores are critical to ion current gating and desalinalion processes insynthetic porous membranes and the functions of biological ion channels. Milethe effects of confinement pore polarizability, and discrete channel chargesites have been much studied, the potentially dramatic impact of dipole-linedsynthetic pores on electrolytes has seldom been addressed. Dipole layersnaturally occur on the interior surfaces of certain nanopores, leading tointrinsic preference for cations or anions. This preference can be exploitedwhen the membrane surface is functionalized differently from the pore interioror when there are alternating dipolar/nondipolar stretches inside a long pore.The dipole-ion interaction is asymptotically unscreened by water, leading toionic, charge segregated, insulating behavior that can block ion transport, andpotentially novel current-voltage (I-V) characteristics.

Ion-dipole interactions are asymptotically unscreened by water in dipolar nanopores, yielding patterned ion distributions