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Thermal and differential thermal analysis techniques, supplemented by microscopic examination of cooled melts, were used to investigate phase equilibrium diagrams for the binary systems: PuCl/sub 3/-MgCl/sub 2/, Pu/Cl/sub 3/ -CaCl/sub 2/, PuCl/sub 3/SrCl/sub 2/, PuCl/sub 3/-BaCl/sub 2/. The PuCl/sub 3/- MgCl/sub 2/ and PuCl/sub 3/-CaCl/sub 2/ systems are characterized by single eutectic points: the PuCl/sub 3/-SrCl/sub 2/ and PuCl/sub 3/-BaCl/sub 2/ systems are characterized by peritectic transformations and solid solutions. Compounds of the tyne M/sub 3/PuCl/sub 9/ (M = Sr or Ba) are associated with the peritectic transformation and solid solutions occur in compositions which are rich in SrCl/ sub 2/ or BaCl/sub 2/.

the journal of physical chemistry

PHASE EQUILIBRIA IN FUSED SALT SYSTEMS: BINARY SYSTEMS OF PLUTONIUM(III) CHLORIDE WITH THE CHLORIDES OF MAGNESIUM, CALCIUM, STRONTIUM AND BARIUM<sup>1</sup>

PHASE EQUILIBRIA IN FUSED SALT SYSTEMS: BINARY SYSTEMS OF PLUTONIUM(III) CHLORIDE WITH THE CHLORIDES OF MAGNESIUM, CALCIUM, STRONTIUM AND BARIUM1

PHASE EQUILIBRIA IN FUSED SALT SYSTEMS: BINARY SYSTEMS OF PLUTONIUM(III) CHLORIDE WITH THE CHLORIDES OF MAGNESIUM, CALCIUM, STRONTIUM AND BARIUM¹