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Laser desorption followed by jet cooling has been used to produce an intense beam of internally cooled benzoic acid monomers. As a result, the SI So gas-phase absorption spectrum of the jet-cooled benzoic acid monomer could be identified for the first time. Delayed ionization out of a triplet state, populated by rapid SI T intersystem crossing, followed by mass-selective detection of the parent ions is performed. The spectral lines have a Lorentzian shape with a line width of 6.5 cm-I, corresponding to an intersystem crossing rate of 1.2 x s-I.

Laser desorption jet-cooling spectroscopy of the benzoic acid monomer