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One-step hydroxylation of benzene to phenol by N2O has been performed over structured catalytic beds made of ZSM-5 coatings on stainless steel grids. The catalysts demonstrated high activity with a selectivity toward phenol formation of 98%. A detailed kinetic study was carried out with a variation in reactant concentrations, benzene/N2O ratio, and residence time. The results obtained suggest a surface reaction between benzene and nitrous oxide adsorbed on two different active sites.

ZSM-5 Coatings on Stainless Steel Grids in One-Step Benzene Hydroxylation to Phenol by N2O: Reaction Kinetics Study

ZSM-5 Coatings on Stainless Steel Grids in One-Step Benzene Hydroxylation to Phenol by N₂O: Reaction Kinetics Study