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Crystal structures of a series of La1-xCexIn3 (x = 0.02, 0.2, 0.5, or 0.8)intermetallic compounds have been investigated by both neutron and X-raydiffraction, and their physical properties have been characterized by magneticsusceptibility and specific heat measurements. Our results emphasize atypicalatomic displacement parameters (ADP) for the In and the rare-earth sites.Depending on the x value, the In ADP presents either an "ellipsoidal"elongation (La-rich compounds) or a "butterfly-like" distortion (Ce-richcompounds). These deformations have been understood by theoretical techniquesbased on the band theory and are the result of hybridization between conductionelectrons and 4f-electrons.

An Experimental and Theoretical Study of the Variation of 4f Hybridization Across the La1-xCexIn3 Series