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Porous poly(ionic liquid)s (PILs) recently have been actively serving as amultifunctional, interdisciplinary materials platform in quite a few researchareas, including separation, catalysis, actuator, sensor, and energy storage,just to name a few. In this context, the capability to photo-pattern PILmicrostructures in a porous state on a substrate is still missing but is acrucial step for their real industrial usage. Here, we developed a method forin situ rapid patterning of porous PIL microstructures via a masklessphotolithography approach coupled with a simple electrostatic complexationtreatment. This breakthrough enables designs of miniaturized sensors. Asexemplified in this work, upon loading Pt nanoparticles into porous PILmicrostructures, the hybrid sensor showed outstanding performance, bearing botha high sensitivity and a wide detection range.

Precise Micropatterning of a Porous Poly(Ionic Liquid) via Maskless Photolithography for High-Performance Non-Enzymatic H2O2 Sensing