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Through the incorporation of a silicon atom to an aryl carboxylic ester substrate, the resulting C-Si bond can be activated via the addition of a carbene catalyst on a remote site. This strategy allows for efficient functionalization of the benzylic sp 3 -carbons of aryl carboxylic esters.

Addition of N-Heterocyclic Carbene Catalyst to Aryl Esters Induces Remote C–Si Bond Activation and Benzylic Carbon Functionalization