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A systematic range of o -hydroxyphenyl ketones were reduced under asymmetric transfer hydrogenation conditions using the C3-tethered catalys 2 . Two directing effects, i.e., an o -hydroxyphenyl coupled to a bulky aromatic on the opposite side of the ketone substrate, combine in a matched manner to deliver reduction products with very high enantiomeric excess.

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Asymmetric Transfer Hydrogenation of <i>o</i>-Hydroxyphenyl Ketones: Utilizing Directing Effects That Optimize the Asymmetric Synthesis of Challenging Alcohols

Asymmetric Transfer Hydrogenation of o-Hydroxyphenyl Ketones: Utilizing Directing Effects That Optimize the Asymmetric Synthesis of Challenging Alcohols