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Shallow donors in ZnO are promising candidates for photon-mediated quantumtechnologies. Utilizing the indium donor, we show that favorable donor-boundexciton optical and electron spin properties are retained in isolated ZnOnanowires. The inhomogeneous optical linewidth of single nanowires (60 GHz) iswithin a factor of 2 of bulk single-crystalline ZnO. Spin initialization viaoptical pumping is demonstrated and coherent population trapping is observed.The two-photon absorption width approaches the theoretical limit expected dueto the hyperfine interaction between the indium nuclear spin and thedonor-bound electron.

Coherent Spin Preparation of Indium Donor Qubits in Single ZnO Nanowires