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Mastery of order-disorder processes in highly non-equilibrium nanostructuredoxides has significant implications for the development of emerging energytechnologies. However, we are presently limited in our ability to quantify andharness these processes at high spatial, chemical, and temporal resolution,particularly in extreme environments. Here we describe the percolation ofdisorder at the model oxide interface LaMnO$_3$ / SrTiO$_3$, which we visualizeduring in situ ion irradiation in the transmission electron microscope. Weobserve the formation of a network of disorder during the initial stages of ionirradiation and track the global progression of the system to full disorder. Wecouple these measurements with detailed structural and chemical probes,examining possible underlying defect mechanisms responsible for this uniquepercolative behavior.

Percolation of Ion-Irradiation-Induced Disorder in Complex Oxide Interfaces