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Most large molecules are chiral in their structure: they exist as twoenantiomers, which are mirror images of each other. Whereas the rovibronicsublevels of two enantiomers are almost identical, it turns out that thephotoelectric effect is sensitive to the absolute configuration of the ionizedenantiomer - an effect termed Photoelectron Circular Dichroism (PECD). Ourcomprehensive study demonstrates that the origin of PECD can be found in themolecular frame electron emission pattern connecting PECD to other fundamentalphotophysical effects as the circular dichroism in angular distributions(CDAD). Accordingly, orienting a chiral molecule in space enhances the PECD bya factor of about 10.

Observation of enhanced chiral asymmetries in the inner-shell photoionization of uniaxially oriented methyloxirane enantiomers