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The theory of catalytic nano-impacts is developed specifically for the case of a single particle in contact with an electrode for a short period of time in which it mediates electron transfer to or from a species in homogeneous solution. The theory is applied to impacts of chemically modified graphene nanoplatelets in which the immobilized ferrocene/ferrocenium couple is used to mediate the oxidation of L-cysteine in aqueous solution. Theory and experiment are in good agreement and the catalytic rate constant is found to be 2.4 ± 1.2 M-1s-

the journal of physical chemistry c

Catalytic Single-Particle Nano-Impacts: Theory and Experiment. Poly(vinylferrocene)-Modified Graphene Nanoplatelet Mediated <scp>l</scp>-Cysteine Oxidation

Catalytic Single-Particle Nano-Impacts: Theory and Experiment. Poly(vinylferrocene)-Modified Graphene Nanoplatelet Mediated l-Cysteine Oxidation