English (United Kingdom)

https://curated-unify.zendy.io/wp-json/zendy-region/v1/featured_content/oa?rat=en

https://curated-unify.zendy.io/wp-json/zendy-region/v1/highlighted_journal/

Global: Zendy Plus annual

Presents the access of premium content as premium feature

Premium Content

Presents the keyphrase highlighting as premium feature

Keyphrase Highlighting

Presents the summarisation as premium feature

Summarisation

Insights

Presents the pdf analysis as premium feature

PDF Analysis

Presents the zaia usage as premium feature

ZAIA

Global: Zendy Plus monthly

Global: Zendy Tools annual

Global: Zendy Tools monthly

Global: Zendy Free Plan

The structure and dynamics of the water/vapor interface is revisited by meansof path-integral and second-generation Car-Parrinello ab-initio moleculardynamics simulations in conjunction with an instantaneous surface definition[A. P. Willard and D. Chandler, J. Phys. Chem. B 114, 1954 (2010)]. Inagreement with previous studies, we find that one of the OH bonds of the watermolecules in the topmost layer is pointing out of the water into the vaporphase, while the orientation of the underlying layer is reversed. Therebetween,an additional water layer is detected, where the molecules are aligned parallelto the instantaneous water surface.

Structure and Dynamics of the Instantaneous Water/Vapor Interface Revisited by Path-Integral and Ab-Initio Molecular Dynamics Simulations