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Direct arylation of thienopyrrolodione, diketopyrrolopyrroles, benzodithiophene derivatives, and fluorinated heteroarenes with functionalized aryl iodides is proven in solvent-free and non-anhydrous conditions. The reaction is performed in the presence of air and tolerates several functional groups on both the coupling partners, enabling a convenient synthesis of extended heteroaromatic conjugated molecules.

Solvent-Free Pd-Catalyzed Heteroaryl–Aryl Coupling via C–H Bond Activation for the Synthesis of Extended Heteroaromatic Conjugated Molecules