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Q-band electron paramagnetic resonance (EPR) data conclusively demonstrate that the iron and cobalt centers in the solid solution [Fe(bpp) 2 ] 0.97 [Co(terpy) 2 ] 0.03 [BF 4 ] 2 (bpp = 2,6-dipyrazol-1-ylpyridine) undergo allosteric spin-state switching during light-induced excited-spin-state trapping (LIESST) at 20 K and thermal relaxation around 80 K. EPR of [Cu(terpy) 2 ] 2+ and [Cu(bpp) 2 ] 2+ , doped into the same host lattice, also indicates expansion of the copper coordination sphere during LIESST excitation.

inorganic chemistry

Interplay between Dopant Species and a Spin-Crossover Host Lattice during Light-Induced Excited-Spin-State Trapping Probed by Electron Paramagnetic Resonance Spectroscopy