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Subhadip Goswami, †,# Jordan N. Nelson, †,# Timur Islamoglu, † Yi-Lin Wu,*∥ Omar K. Farha,*∥ and Michael R. Wasielewski*∥ † Department of Chemistry, Northwestern University, Evanston, Illinois 60208, United States  §Argonne−Northwestern Solar Energy Research (ANSER) Center, Northwestern University, Evanston, Illinois 60208, United States ∥Institute for Sustainability and Energy at Northwestern (ISEN), Northwestern University, Evanston, Illinois 60208, United States  ‡ Department of Chemistry, Faculty of Science, King Abdulaziz University, Jeddah 22254, Saudi Arabia

Photoexcited Naphthalene Diimide Radical Anion Linking the Nodes of a Metal–Organic Framework: A Heterogeneous Super-reductant