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We present a comprehensive study of the adsorption behavior of ironphthalocyanine on the low-index crystal faces of silver. By combiningmeasurements of the reciprocal space by means of photoelectron momentum mappingand low energy electron diffraction, the real space adsorption geometries arereconstructed. At monolayer coverage ordered superstructures exist on allstudied surfaces containing one molecule in the unit cell in case of Ag(100)and Ag(111), and two molecules per unit cell for Ag(110). The azimuthal tiltangle of the molecules against the high symmetry directions of the substrate isderived from the photoelectron momentum maps. A comparative analysis of themomentum patterns on the substrates with different symmetry indicates that bothconstituents of the twofold degenerate FePc lowest unoccupied molecular orbitalare occupied by charge transfer from the substrate at the interface.

Adsorption geometry and electronic structure of iron phthalocyanine on Ag surfaces: A LEED and photoelectron momentum mapping study