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Epitaxial heterostructures of La0.6Sr0.4MnO3 0.7Pb(Mg0.33Nb0.67)O3 0.3PbTiO3were fabricated on LaNiO3 coated LaAlO3 (100) substrates by pulsed laserablation. Ferromagnetic and ferroelectric hysteresis established theirbiferroic nature. Dielectric behviour studied under different magnetic fieldsover a wide range of frequency and temperatures revealed that the capacitancein these heterostructures varies with the applied magnetic field. Appearance ofmagnetocapacitance and its dependence on magnetic fields, magnetic layerthickness, temperature and frequency indicated a combined contribution ofstrain mediated magnetoelectric coupling, magnetoresistance of the magneticlayer and Maxwell Wagner effect on the observed properties.

Magnetocapacitive La0.6Sr0.4MnO3 0.7Pb(Mg0.33Nb0.67)O3 0.3PbTiO3 epitaxial heterostructures