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During the solidification of Al-Sm metallic glasses the evolution of thesupercooled liquid atomic structure has been identified with an increasingpopulation of icosahedral-like clusters with increasing Sm concentration. Theseclusters exhibit slower kinetics compared to the remaining clusters in theliquid leading to enhanced amorphous phase stability and glass forming ability(GFA). Maximum icosahedral-ordering and atomic packing density have been foundfor the Al90Sm10 and Al85Sm15 alloys, respectively, whereas minimum cohesiveenergy has been found for the Al93Sm7 which is consistent with the range ofcompositions (from Al92Sm8 to Al84Sm16) found experimentally with high GFA.

On the role of Sm in solidification of Al-Sm metallic glasses