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We study the dynamics of multiple coupled states under the influence of anarbitrary time-dependent external field to investigate the femtosecondlaser-driven excitation and the spin-orbit mediated dissociation in the NaRbdimer. In this process, the dimer is excited from the ground triplet state$1^3\Sigma^+$ to the $1^3\Pi$ state using the femtosecond laser impulse and thespin-orbit coupling between the $1^3\Pi$ and $2^1\Sigma^+$ states results inthe singlet-triplet transition. The laser impulse parameters are optimised toobtain maximum yield in electronic states correlating with the first excitedatomic asymptote. We observe the detailed population statistics and power-lawdecay of these states. Finally, the analysis of the population oscillationsallows us to determine the optimal time delay for dumping the molecule to itsabsolute ground state.

Optimization of the Femtosecond Laser Impulse for Excitation and the Spin-Orbit Mediated Dissociation in the NaRb Dimer