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Spectral bands for the B(2)$^{2}\Sigma^{+}\rightarrow$ X(1)$^{2}\Sigma^{+}$electronic transition in the doubly-polar open-shell KSr molecule are recordedat moderate resolution using the thermoluminescence technique. The spectra aresimulated using three kinds of advanced electronic structure calculations,allowing for an assessment of their accuracy on one hand, and for thederivation of fundamental spectroscopic constants of the X(1)$^{2}\Sigma^{+}$KSr ground state and the excited electronic state B(2)$^{2}\Sigma^{+}$, on theother hand. These results should facilitate further studies aiming at creatingultracold bosonic or fermionic KSr molecules.

Experimental and theoretical study of the B(2)$^2 \Sigma^+ \rightarrow$ X(1)$^2 \Sigma^+$ system in the KSr molecule