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In this study, we determined the different physical characteristics ofnanoscale layered mixed Fe-Co layers of orthoferrite SmFe0.5Co0.5O3 based onmagnetic and dielectric measurements.Magnetization analyzes showed that thesystem was antiferromagnetic with a magnetic transition around 310 K and twospin-reorientation transitions at around 192 K and 22 K.In this phase, theantisymmetric exchange interaction induced weak ferromagnetism due to cantingof the magnetic spins in a similar manner to the Ln-Fe-Co system. Importantly,this nanoscale layered perovskite also exhibited a positive magneto-dielectriceffect of around 2.5 % (100 K) and the value decreased on both sides of thistemperature.We analyzed the conditions related to the existence of magnetic anddielectric coupling in terms of the magnetic interactions between the cationsas well as the spin-lattice interactions in the low temperature range.

Low temperature Magneto-dielectric coupling in nanoscale layered SmFe0.5Co0.5O3 perovskite