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Diverse polymer crosslinking techniques allow the synthesis of linearpolymer-like structures whose monomers are colloidal particles. In the casewhere all or part of these colloidal particles are magnetic, one can controlthe behaviour of these supracolloidal polymers, known as magnetic filaments(MFs), by applied magnetic fields. However, the response of MFs stronglydepends on the crosslinking procedure. In the present study, we employ Langevindynamics simulations to investigate the influence of the type of crosslinkingand the distribution of magnetic particles within MFs on their response to anexternal magnetic field. We found that if the rotation of the dipole moment ofparticles is not coupled to the backbone of the filament, the impact of themagnetic content is strongly decreased.

journal of magnetism and magnetic materials

The influence of crosslinkers and magnetic particle distribution along  the filament backbone on the magnetic properties of supracolloidal linear  polymer-like chains