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The crystalline garnet Mn3Fe2Si3O12 and an amorphous phase of the samenominal composition are synthesized at high pressure. The magnetic propertiesof the two forms are reported. Both phases order antiferromagnetically. Thecrystalline phase exhibits a Curie-Weiss theta of -47.2 K, with a sharpordering transition at 12 K. The glassy phase exhibits a largerantiferromagnetic Curie-Weiss theta, of -83.0 K, with a broad orderingtransition observed at 2.5 K. Both phases can be classified as magneticallyfrustrated, although the amorphous phase shows a much higher degree offrustration. The amorphous phase exhibits spin-glass behavior and is determinedto have an actual composition of Mn3Fe2Si3O13.

Comparison of the Magnetic properties of Mn3Fe2Si3O12 as a crystalline garnet and as a glass