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Mn3TeO6 exhibits a corundum-related A3TeO6 structure and a complex magneticstructure involving two magnetic orbits for the Mn atoms [*]. Mn3-xCdxTeO6(x=0, 1, 1.5 and 2) ceramics were synthesized by solid state reaction andinvestigated using X-ray powder diffraction, electron microscopy, calorimetricand magnetic measurements. Cd2+ replaces Mn2+ cations without greatly affectingthe structure of the compound. The Mn and Cd cations were found to be randomlydistributed over the A-site. Magnetization measurements indicated that thesamples order antiferromagnetically at low temperature with a transitiontemperature that decreases with increasing Cd doping. The nuclear and magneticstructure of one specially prepared 114Cd containing sample:Mn1.5(114Cd)1.5TeO6, was studied using neutron powder diffraction over thetemperature range 2 to 295 K. Mn1.5(114Cd)1.5TeO6 was found to order in anincommensurate helical magnetic structure, very similar to that of Mn3TeO6 [*].However, with a lower transition temperature and the extension of the orderedstructure confined to order 240(10) {\AA}. [*] S. A. Ivanov et al. Mater. Res.Bull. 46 (2011) 1870.

Structural and magnetic properties of Mn3-xCdxTeO6 (x = 0, 1, 1.5 and 2)