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Structures resembling semiclathrates probably arise in liquid aqueoussolutions of piperidine at the amine mole fraction below 0.03. With theincreasing concentration, the structures gradually decay, but the 1:1 complexesof piperidine with water remain linked one to another through the O-H...O bondsbetween the hydration water molecules. A periodic order of the bicontinuousmicroemulsion type occurs in the range of the mole fractions from 0.08 to 0.5.In the piperidine-rich mixtures, the 1:1 complexes are dispersed uniformly inthe amine. Relatively low stabilization energy of these complexes probablycauses that piperidine is totally miscible with water.

Hydrogen-bonded aggregates in the mixtures of piperidine with water: thermodynamic, SANS and theoretical studies