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The search for materials displaying a large magnetoelectric effect hasoccupied researchers for many decades. The rewards could include not onlyadvanced electronics technologies, but also fundamental insights concerning thedielectric and magnetic properties of condensed matter. In this article, wefocus on the magnetoelectric effect in transition metal oxides and review themanner in which first-principles calculations have helped guide the search for(and increasingly, predicted) new materials and shed light on the microscopicmechanisms responsible for magnetoelectric phenomena.

The Magnetoelectric Effect in Transition Metal Oxides: Insights and the Rational Design of New Materials from First Principles