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Two-dimensional chromium oxide fluoride CrOF sheet was studied based ondensity functional theory. The investigation indicates that the CrOF sheet isan intrinsic ferromagnetic semiconductor. The calculated low cleavage energyimplies that the ferromagnetic semiconductor can be exfoliated from its bulkform. The corresponding Curie temperature is 150 K. In particular, the Curietemperature increases up to 410 K under hole doping and the CrOF sheet becomesa half-metal. The versatile electronic and magnetic properties indicate thatthe two-dimensional CrOF sheet can be a promising candidate for next-generationspintronic devices.

Theoretical prediction of two-dimensional CrOF sheet as a ferromagnetic semiconductor or a half-metal