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Bi 2 Sr 2−x Cs x Co 2 O y  materials with 0 ≤ x ≤ 0.15, have been fabricated via the classical ceramic technique. XRD results have indicated that undoped and Cs-substituted samples are composed of Bi 2 Sr 2 Co 2 O y  phase as the major one. Microstructural studies have demonstrated the formation of a liquid phase, which allows a drastic grain growth. This factor is responsible for a drastic improvement of relative density, reaching about 95% of the theoretical one for 0.125 Cs content. On the other hand, electrical resistivity has been reduced up to 14 mΩ cm at 650 °C for 0.125 Cs content, around 40% lower than the obtained in undoped samples. As a consequence, Seebeck coefficient has been decreased due to the raise in charge carrier concentration. The highest power factor at 650 °C (0.21 mW/K 2  m) has been found for 0.125 Cs substituted sample, about 40% larger than the obtained in undoped samples, and very similar to the notified in single crystals (0.26 mW/K 2  m). Magnetisation with respect to temperature results have demonstrated that measured samples have a paramagnetic property above 50 K, except 0.10 Cs. Magnetic hysteresis curves have shown that the slopes and the magnitudes have increased with decreasing temperature.

Detail investigation of thermoelectric performance and magnetic properties of Cs-doped Bi2Sr2Co2Oy ceramic materials