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HighlightsA three-dimensional spider web-inspired structured graphene skeleton is constructed.    The spider web-like skeleton endows paraffin wax with a significantly high longitudinal and transverse thermal conductivity enhancement of ~1260% and ~840%, respectively, at 2.25 vol% skeleton.    The resultant composites exhibit outstanding performance on the thermal management of Li-ion batteries.Supplementary Information  The online version contains supplementary material available at 10.1007/s40820-021-00702-7.

Spider Web-Inspired Graphene Skeleton-Based High Thermal Conductivity Phase Change Nanocomposites for Battery Thermal Management