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HighlightsUltra-thin CoNiO 2  nanosheet with rich oxygen defects anchored on the vertically arranged Ni nanotube arrays (O d -CNO@Ni NTs) is successfully constructed.    The O d -CNO@Ni NTs electrode delivers extraordinary electrochemical performance.    The theoretical calculations reveal that oxygen defects effectively improve the electrochemical kinetics and the surface electronic state structure of O d -CNO @ Ni NTs, thus exhibiting strong OH  −  adsorption capacity.Supplementary Information  The online version contains supplementary material available at 10.1007/s40820-021-00699-z.

Oxygen-Defect Enhanced Anion Adsorption Energy Toward Super-Rate and Durable Cathode for Ni–Zn Batteries