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HighlightsThe delicate “3D helix–2D sheet–1D fiber–0D dot” hierarchical aerogels were successfully synthesized.    The graphene sheets are uniformly intercalated by helical carbon nanocoils, which endow the as-obtained aerogel with abundant porous structures and better dielectric properties.    By adjusting the growth parameters of 0D core-shell structured particles and 1D carbon nanofibers, the tunable electromagnetic properties and excellent impedance matching are achieved.Supplementary Information  The online version contains supplementary material available at 10.1007/s40820-021-00667-7.

nano-micro letters

Structural Engineering of Hierarchical Aerogels Comprised of Multi-dimensional Gradient Carbon Nanoarchitectures for Highly Efficient Microwave Absorption