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HighlightsA newly versatile self-sacrifice method to fabricate selenium and nitrogen co-doped 3D macroporous carbon was developed.    The K +  storage mechanism of Se and N active sites was deeply studied by systematic electrochemical characterization combined with theoretical calculations.    The assembled K-ion hybrid capacitor possesses high energy/power densities and excellent cycling stability for practical applications.Supplementary Information  The online version contains supplementary material available at 10.1007/s40820-021-00659-7.

A General Self-Sacrifice Template Strategy to 3D Heteroatom-Doped Macroporous Carbon for High-Performance Potassium-Ion Hybrid Capacitors