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HighlightsThe unique wire-in-wire structure endows TiO 2 /C nanofibers film with superior mechanical flexibility.    The wire-in-wire TiO 2 /C nanofibers (TiO 2  ww/CN) film shows outstanding electrochemical performances as free-standing anodes for Li/K-ion batteries and full cells.    The TiO 2  ww/CN film shows an extremely high pseudocapacitance contribution ratio in K-ion batteries.Supplementary Information  The online version contains supplementary material available at 10.1007/s40820-021-00632-4.

Wire-in-Wire TiO2/C Nanofibers Free-Standing Anodes for Li-Ion and K-Ion Batteries with Long Cycling Stability and High Capacity