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HighlightsN-doped graphene-coated structure and mesoporous nano-sheet can efficiently boost active sites and stability for hydrogen and oxygen evolution reaction.    NiCo@C-NiCoMoO/NF exhibits low overpotentials for HER (266 mV) and OER (390 mV) at ± 1000 mA cm −2 .    For water electrolysis, it can hold at 1000 mA cm −2  for 43 h in 6.0 M KOH + 60 °C condition.Supplementary Information  The online version contains supplementary material available at 10.1007/s40820-021-00607-5.

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N-Doped Graphene-Decorated NiCo Alloy Coupled with Mesoporous NiCoMoO Nano-sheet Heterojunction for Enhanced Water Electrolysis Activity at High Current Density