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HighlightsThe sensors displayed high sensitivity (8962.7), fast response time (60 ms), outstanding stability and durability (> 10,000 cycles) and widely workable stretching range (0–160%).    A theoretical approach was used to analyze mechanical property, and a model based on tunneling theory was modified to describe the relative change of resistance.    Two equations were proposed and offered an effective but simple approach to analyze the change of number of conductive paths and distance of adjacent conductive particles.Supplementary information  The online version of this article (10.1007/s40820-021-00592-9) contains supplementary material, which is available to authorized users.

Highly Sensitive Ultrathin Flexible Thermoplastic Polyurethane/Carbon Black Fibrous Film Strain Sensor with Adjustable Scaffold Networks