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HighlightsA facile strategy is proposed to construct novel CoO and NiO electrode material with interior (Cu + ) and exterior (metallic Cu 0 ) decoration for supercapacitor.    The co-doped CoO electrode presents four times higher specific capacitance and more cycle stability than that of pristine CoO.    The conductivity and electron transport rate of CoO with Cu 0 /Cu +  co-doping have been effectively improved and confirmed by detailed theoretical calculations.Supplementary information  The online version of this article (10.1007/s40820-021-00590-x) contains supplementary material, which is available to authorized users.

Interior and Exterior Decoration of Transition Metal Oxide Through Cu0/Cu+ Co-Doping Strategy for High-Performance Supercapacitor