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HighlightsThe ultrathin nickel metal–organic framework (MOF) nanosheets in situ interpenetrated by functional carboxylated carbon nanotubes (C-CNTs) were successfully constructed. The incorporated C-CNTs effectively adjust the layer thickness of Ni-MOF nanosheets.    The integrated hybrid MOF nanosheets delivered the boosted electrochemical performances and exhibited superior specific capacity of 680 C g −1  at 1 A g −1 .Electronic supplementary material  The online version of this article (10.1007/s40820-020-0382-x) contains supplementary material, which is available to authorized users.

Ultrathin 2D Metal–Organic Framework Nanosheets In situ Interpenetrated by Functional CNTs for Hybrid Energy Storage Device