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HighlightsThe ultrathin metal–organic-framework (MOF) interphase layer with high mechanical/chemical stability was in situ grown on black phosphorus nanosheets (BPNSs).    MOF interphase layers as an ordered porous and robust protective layer can facilitate K ion diffusion and accommodate the volume change of the electrode.    Benefiting from the improved reaction kinetics and enhanced electrode stability, the BPNS@MOF anode for potassium-ion capacitors exhibits outstanding cycle performance.Electronic supplementary material  The online version contains supplementary material available at (10.1007/s40820-020-00570-7) contains supplementary material, which is available to authorized users.

Armoring Black Phosphorus Anode with Stable Metal–Organic-Framework Layer for Hybrid K-Ion Capacitors