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HighlightsModerate-concentration ZnCl 2  (15 m) was found to be effective for suppressing the dissolution of vanadate cathode, which was more stable and had 4 times higher ionic conductivity than 30 m “water-in-salt” electrolyte.    K 0.486 V 2 O 5  with huge interlayer space of ~ 0.95 nm was chosen for the first time to assemble aqueous Zn ion batteries, giving rise to excellent rate performance and high energy and power densities.    A novel sodium carboxymethyl cellulose-15 m ZnCl 2  hydrogel electrolyte with high ionic conductivity of 10.08 mS cm −1  was designed, enabling a bendable Zn ion battery with outstanding resistance to temperature and pressure.Electronic supplementary material  The online version of this article (10.1007/s40820-020-00554-7) contains supplementary material, which is available to authorized users.

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Electrolyte Concentration Regulation Boosting Zinc Storage Stability of High-Capacity K0.486V2O5 Cathode for Bendable Quasi-Solid-State Zinc Ion Batteries