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Highlights3D Zn-doped CuO framework was designed for aligned distributing high mass loading of MnO 2  nanosheets.    Zn could be introduced into the CuO crystal lattice to tune the covalency character and thus improve charge transport.    A free-standing asymmetric coaxial fiber-shaped supercapacitor based on Zn–CuO@MnO 2  core electrode possesses superior performance including higher capacity and better stability under deformation.Electronic supplementary material  The online version of this article (10.1007/s40820-020-00529-8) contains supplementary material, which is available to authorized users.

Atomic Modulation of 3D Conductive Frameworks Boost Performance of MnO2 for Coaxial Fiber-Shaped Supercapacitors