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HighlightsRhodium ion incorporation helps the nucleation of perovskite grain, passivates the defects in the grain boundaries and enhances the film quality, charge carrier lifetime and mobility.    After optimizing 1% rhodium into perovskite film, the solar cells achieve an efficiency of 20.71% without obvious hysteresis.Electronic supplementary material  The online version of this article (10.1007/s40820-020-00457-7) contains supplementary material, which is available to authorized users.

Perfection of Perovskite Grain Boundary Passivation by Rhodium Incorporation for Efficient and Stable Solar Cells