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HighlightsMicroporous indium-based metal–organic framework (In-BTC) nanocrystals are synthesized under an extremely mild condition.    Perovskite/In-BTC heterojunction films possess improved morphology/crystallinity and reduced grain boundaries/defects.    In-BTC-modified perovskite solar cells exhibit significantly enhanced efficiency of 20.87% and long-term stability.Electronic supplementary material  The online version of this article (10.1007/s40820-020-00417-1) contains supplementary material, which is available to authorized users.

Heterojunction Incorporating Perovskite and Microporous Metal–Organic Framework Nanocrystals for Efficient and Stable Solar Cells