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HighlightsVarious forms of carbon nanomaterials are selected as substrates to clear the mist in understanding the reactivity/utility of ferrate(VI) in oxidizing carbon nanomaterials.    It unravels a modest reactivity of ferrate(VI) in liquid phase that only oxidizes the active defects on carbon surface and a powerful oxidizing ability in solid state that can open the inert C=C bonds in carbon lattice.    Respective benefit and limitation of the wet and dry approaches using ferrate(VI) in functionalizing carbon nanomaterials are discussed.Electronic supplementary material  The online version of this article (10.1007/s40820-019-0353-2) contains supplementary material, which is available to authorized users.

Versatile Functionalization of Carbon Nanomaterials by Ferrate(VI)