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HighlightsFe 1− x  S/MoS 2  heterostructure with abundant “ion reservoir” interfaces is designed to reduce sodium ion diffusion barrier and facilitate charge-transfer kinetics, thus endowing the electrode with excellent cycling stability and rate capability.    The in-depth analysis on the dynamic relationship between heterointerface and sodium storage performance carves a new path for interface engineering toward the next-generation high-performance energy storage devices.Electronic supplementary material  The online version of this article (10.1007/s40820-019-0311-z) contains supplementary material, which is available to authorized users.

Boosting Sodium Storage of Fe1−xS/MoS2 Composite via Heterointerface Engineering