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HighlightsWe first report on H 11 Al 2 V 6 O 23.2  with large layer spacing as cathode for aqueous zinc-ion battery, which accelerates the diffusion of Zn 2+ .    The graphene-wrapped H 11 Al 2 V 6 O 23.2  nanobelts can improve electronic conductivity, and potentially inhibit the dissolution of elements in the aqueous electrolyte.    H 11 Al 2 V 6 O 23.2 @graphene exhibits high capacity and stable cycling stability even at an ultra-high mass loading of ~ 15.7 mg cm −2 .Electronic supplementary material  The online version of this article (10.1007/s40820-019-0300-2) contains supplementary material, which is available to authorized users.

Ultra-High Mass-Loading Cathode for Aqueous Zinc-Ion Battery Based on Graphene-Wrapped Aluminum Vanadate Nanobelts