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HighlightsFacile electrodeposition for fabricating active Ni nanodots (NiNDs) on Ni foam (NF) is shown.    Binder- and heteroatom-free recyclable NiO/NiNDs@NF electrodes are efficiently made.    NiO/NiNDs@NF bifunctional catalytic electrodes are used for water splitting.Electronic supplementary material  The online version of this article (10.1007/s40820-019-0269-x) contains supplementary material, which is available to authorized users.

Prompt Electrodeposition of Ni Nanodots on Ni Foam to Construct a High-Performance Water-Splitting Electrode: Efficient, Scalable, and Recyclable