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Highlights2D Mo 2 C was produced by a modified chemical vapor deposition method, and 2D Mo 2 C-Au was formed as an asymmetric contact structure with a large work function difference.    Mo 2 C/MoS 2 /Au photodetectors powered by asymmetric contact structure can work under self-powered condition with a responsivity of 10 −1  mA W −1 . The detection performance of the photodetectors can be stable for at least 110 days.Electronic supplementary material  The online version of this article (10.1007/s40820-019-0262-4) contains supplementary material, which is available to authorized users.

MoS2-Based Photodetectors Powered by Asymmetric Contact Structure with Large Work Function Difference