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HighlightsAn effective in situ coupling strategy is proposed to construct Co 9 S 8  nanoparticles/doped graphene.    Cobalt porphyrin derivative is employed as both coupling and heteroatom-doped agents.    The bifunctional oxygen electrocatalyst finds application in rechargeable all-solid-state Zn–air batteries.Electronic supplementary material  The online version of this article (10.1007/s40820-018-0231-3) contains supplementary material, which is available to authorized users.

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In Situ Coupling Strategy for Anchoring Monodisperse Co9S8 Nanoparticles on S and N Dual-Doped Graphene as a Bifunctional Electrocatalyst for Rechargeable Zn–Air Battery